As I sort of expected, the "Best of Dan Decarlo" collection doubles as a "Best of Frank Doyle", and focuses in on 1958 through the 1960s -- up to, I guess, when "Archies" mania punched out some of the quality of the Archies.

My sense is that this cannot stand as is. There are other stories to republish and call "Best", from different eras.
A run down of stories. Off the top of my mind, I'm familiar with a few of these -- "The Midas Mess", for instance. Of those I don't recognize, I suggest that this is pretty intriguing:

17. “Bully Girl” (Betty and Veronica # 106) – Veronica shows off her new martial arts skills by beating up everyone in sight.

As I've said before, Give me the Best of Samm Schwartz -- which I don't think can be ecapsuled in one era quite as well as Decarlo probably can, and then you'll have me.